Study of a Nuclear Resonance in the Reaction 19F(p,a g )16O.

Read K.S. Krane chapter 11 about nuclear reactions up to 11.13 Heavy-Ion Reactions. Also read chapter 15 about beam handling and electrostatic accelerators.

Accelerators, general background

Ernest Rutherford made experiments where he used energetic alpha particles which he obtained from a radioactive source. He let alpha particles hit a gold foil and observed how they were scattered. These experiments showed that the main part of the mass of the atom was concentrated to the centre of the atom. Eventually these findings led Niels Bohr to create a new model for the atom.

However in the long run it's neither very "healthy" nor "flexible" to use strong radioactivity as source of energetic alpha particles. Therefore some persons started to think about how to accelerate ions to high velocities artificially. The very first accelerator in which ions could be accelerated to energies high enough to induce nuclear reactions was built 1930 by Cockroft and Walton This accelerator was a linear accelerator and the principle to create a high energy was based on cascade generation of high voltage. At about the same time Ernest Lawrence had started to think in another direction. He invented the cyclotron. He and M. Stanley Livingstone built the first at Berkeley 1931.

Swedish scientists became highly interested in the new physics that was emerging during the first decades of the century. According to some unofficial sources two Nobel prizes (one in physics and one in chemistry) were "confiscated" and used to create the Nobel Institute of Physics. Manne Siegbahn became the first director of this institute and his first task was to build a cyclotron. (Today what's remaining of the former Nobel Institute of Physics is called the Manne Siegbahn Laboratory and that's where this laboration takes place).

The cyclotron was ready during autumn 1939. With it protons, deuterons and alpha particles could be accelerated. Cyclotrons are often characterised by their pole diameter. It tells to what energy particles can be accelerated for a given magnetic field strength. The cyclotron of the Nobel Institute had a diameter of 80 cm.

Already 1944 Manne Siegbahn presented plans to build a bigger cyclotron. Within half a year he received 500000 Swedish kronor from the Rockefeller foundation in USA. This money was enough to start a project to build a 225 cm cyclotron. Hard labour and economical grants from the Knut and Alice Wallenberg foundation, the Nobel foundation and the government made it possible to reach the goal; deuterons accelerated to 25 MeV, already in autumn 1951.

The 225 cm cyclotron was a "classical" cyclotron working at a fixed frequency. The frequency had to be set for each ion and experiment and could not be varied in short time. This meant that one could not adjust the frequency when ions became relativistic. Another limiting factor was that the ion sources that were placed at the centre of the cyclotron could not produce highly charged ions. This limited the ions that could be accelerated to be lighter or equal to oxygen. Gradually it became evident that the institute needed a new accelerator and during the end of the 80s a new accelerator project was started. On the day of St Lucia 1990 we had our first ion beam circulating in our new accelerator and storage ring CRYRING 1990. Today it's used for atomic and molecular physics studies and for applications like the testing of micro electronics circuits for outer space and other surroundings with intense radiation. Today accelerator techniques are used in many fields of physics and also for applications of many kinds.

About the accelerator we are using.

Since the very beginning the institute also had smaller accelerators. The accelerator we are using to make nuclear reactions is a single ended Van de Graaff. It's a linear accelerator and the accelerating voltage is obtained by charging a rubber belt, which in turn charges the so-called terminal. You have probably seen a small desktop version of a Van de Graaff during your studies of physics. Our Van de Graaff can be charged to a maximum voltage of about 2.5 MV. Singly charged ions can therefore reach a maximum of 2.5 MeV. An ion with charge 2+ can consequently reach 5 MeV.

In a tandem Van de Graaff negative ions are injected at the low energy end and are accelerated towards the terminal which is charged to a voltage V. Inside the terminal, the singly charged ions have reached V eV. The relatively high energy at the terminal is utilised to strip off a number of electrons = q. This is done with a thin carbon foil or a gas at low pressure. On the way out the ions thereafter gain an energy of qV eV and reach a total energy of (q+1)V eV.

Our single ended Van de Graaff is equipped with a radio frequency ion source in the terminal. The ion source is fed with gases like H2 or mixtures of 3He and 4He. The ion source can be remotely controlled.

Nuclear reactions.

In the following we will describe nuclear reactions from a general point of view. After that we will consider a few important aspects of nuclear reactions.

A nuclear reaction between a projectile nucleus x and a target nucleus X might result in one or more new nuclei. Here we consider production of two new nuclei y and Y and we write the nuclear reaction as:

x + X ® Y + y

One can also write X(x,y)Y to describe the same reaction. If y = x and Y = X we call what has happened "scattering".

At low projectile energy only electromagnetic interactions play a role. Since nuclei in our world all are positively charged they are repelling each other by Coulomb forces. At higher energy when the projectile "touches" the target nucleus the strong force start to play a role. A simple estimate of how much energy is needed to overcome the Coulomb repulsion can be obtained if one considers the projectile and target nuclei as two charged spheres.

The following 5 tasks should be done in advance.

Task 1: Calculate the kinetic energy which is required to overcome the repulsive energy at a distance between two spheres representing a proton and a 19F nucleus. Use reasonable estimates of the radii of the proton and the 19F nucleus.

Another important property in nuclear reactions is the equivalence of energy and mass. The Q-value is defined by equation 11.2 in Krane, here numbered (1)

 

where M and m are masses, indices refer to the formulas above and Ts are kinetic energies of respective particles. c is of course the speed of light.

The Q-value is important because it tells us how much energy is available or needed for the reaction to take place. If Q> 0 energy is released in the reaction and this energy is shared as kinetic energy by the two new nuclei.

The kinetics of a nuclear reaction can be calculated if one knows the initial energy of the projectile and the masses of the initial and final nuclei involved in the reaction.

Task 2: Calculate the Q-values of the reactions:

p + 19F ® 20Ne and p + 19F ® 16O + a

20Ne is the so-called compound nucleus. The compound nucleus is an intermediate step in compound nuclear reactions.

In this laboratory exercise we are going to study a resonance in the scattering of protons against 19F. The nuclear reaction is described by the formula 19F (p,a g ) 16O. A resonance occurs at a specific kinetic energy of the proton beam matching the energy of a specific state in the compound nucleus. By calculation of the Q-value one can get an estimate of the energy that is available when forming 20Ne and learn which level might be responsible for the resonance we are studying.

Task 3: Study the level scheme of 20Ne. Is it possible to find out which level that can cause the observed resonance?

Task 4: Study the level scheme of 16O and discuss what gamma transition energies one can expect to see in this reaction.

Task 5: Use the equation below to calculate the energy of a -particles and 16O ions detected at 170o with respect to the beam direction. How do you cope with the fact that 16O can be produced in an excited state? For an explanation of the variables of the equation look up equation (11.5) of Krane, here numbered (2).

 

Detectors:

In order to study nuclear reactions detectors for different kind of radiation are used. In this laboratory exercise we use a silicon surface barrier detector to detect the alpha particle that is one product of the reaction. The silicon detector is placed at an angle of 170o with respect to the beam direction. We further use a high purity germanium detector to observe gamma transitions in the nucleus 16O. The compound nucleus does not live long enough to emit discrete gamma transitions. If you look at the level scheme of 16O you see that the gamma transitions that can be expected are of quite a high energy. We have no calibration sources for gamma transitions of very high energy. However in a house with basement concrete is the most common building material. In concrete there are a few gamma transitions belonging to the normal radioactive background.

Experimental tasks:

  1. Calibration of the surface barrier detector by means of a calibrated alpha source.
  2. The calibration source contains 3 alpha emitting radioactive isotopes: 239Pu, 241Am and 244Cm. These sources have the following a -energies (in MeV) and relative intensities (in %).

    Radioactive

    Isotopes Þ

    239Pu

    241Am

    244Cm

    Alpha

    5.082 0.03

    5.389 1.3

    5.764 23.3

    Particle

    5.111 11.5

    5.443 12.8

    5.806 76.7

    Energies Þ

    5.142 15.1

    5.486 85.2

     

    and

    5.161 73.3

    5.513 0.12

     

    Intensities

     

    5.544 0.35

     

    This information can also be used to determine the resolution of the silicon detector (including noise etc from the electronic system).

  3. Calibration of the germanium detector. Find the "background" gamma transitions and identify these. A preliminary calibration is done with a source of 22Na.
  4. Experimentally record the resonance at 1.372 MeV in the nuclear reaction 19F(p,g a )16O. The energy of the proton beam is varied. The resonance is monitored by counting the number of detected alpha particles as well as the number of detected gamma quanta belonging to transitions in 16O. Take as many energy "points" as necessary to get an estimate of the half-width of the resonance. The "points" are normalised by integration of the measured beam current. That gives the total charge collected during each measured point. Can you detect 16O directly in the silicon detector?

Questions to address during the experiment:

Which "phenomena or parameters" might influence the width of the "peak" in the spectrum of the Si-detector?

Which "phenomena or parameters" might influence the width of the resonance? Find the half-width of the resonance. Estimate the lifetime of the resonant state.

Identify the states of 16O populated in the reaction by studying the a -particle and g -ray spectra. You might need to compare spectra obtained at a proton energy at resonance as well as below resonance.

Are the a -particle energies in agreement with eq. (2)?

Importance of nuclear reactions, some subjects to study further:

Astrophysically important reactions in nucleo-synthFigure 1esis.

Reactions related to production of energy by fusion of nuclei.

Elemental analysis by means of nuclear reactions.

Fig. 1

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Fig. 4